Rechargeable all-solid-state batteries (ASSBs) comprising solid electrodes and electrolytes have attracted significant interest as next-generation battery systems because of their high energy density and enhanced safety, as compared to conventional lithium-ion battery (LIBs). However, numerous challenges, such as poor ionic conductivity of the solid electrolyte (SE), dendrite formation, unstable solid-solid interface between the electrolyte and electrodes, and limited cycle life, impede the industrial commercialization of ASSBs. 2D MXenes have recently emerged as advanced electrode and electrolyte materials capable of addressing the technical challenges faced by ASSBs owing to their unique properties such as outstanding metallic conductivity, abundant surface terminations, and metal-ion-philic surface properties. This review summarizes the latest advancements in MXene-based ASSB research for lithium, sodium, and zinc batteries. Furthermore, the technical challenges of MXene-based ASSBs are discussed and future perspectives and potential directions for the development of MXene-based ASSBs for next-generation energy storage systems are proposed.
Bibliographical noteFunding Information:
This study was supported by grants from the Basic Science Research Program ( 2021M3H4A1A03047327 and 2022R1A2C3006-227 ) through the National Research Foundation of Korea , funded by the Ministry of Science, ICT, and Future Planning; the Fundamental R&D Program for Core Technology of Materials and the Industrial Strategic Technology Development Program ( 20020855 ), funded by the Ministry of Trade, Industry, and Energy, Republic of Korea. This study was also partially supported by a grant (CRC22031-000) from Korea Institute of Science and Technology and the National Research Council of Science & Technology (NST) , funded by the Korean Government (MSIT) . Furthermore, this study was partially supported by a start-up fund (S-2022-0096-000) and the Postdoctoral Research Program of Sungkyunkwan University (2022).
© 2023 Elsevier Ltd
- 2D MXenes
- All-solid-state batteries
- Dendrite free surface
- Energy density
- Ionic conductivity
- Solid-state electrolytes
ASJC Scopus subject areas
- Renewable Energy, Sustainability and the Environment
- Materials Science (miscellaneous)
- Nuclear Energy and Engineering
- Fuel Technology
- Energy Engineering and Power Technology