Highly sensitive and long-term stretchable eutectic nanogel conductor with conducting interpenetrating nanogel networks for monitoring human motions

Jun Ho Lim; Min Jeong Kim; Ho Gyu Yoon; Sang Woo Kim

doi:10.1016/j.compositesb.2022.110299

Highly sensitive and long-term stretchable eutectic nanogel conductor with conducting interpenetrating nanogel networks for monitoring human motions

Jun Ho Lim, Min Jeong Kim, Ho Gyu Yoon, Sang Woo Kim

Research output: Contribution to journal › Article › peer-review

14 Citations (Scopus)

Abstract

As a stretchable e-skin for sensing repetitive and stressful body movements, we photo-polymerized choline chloride─acrylic acid (CA) deep eutectic solvents (DESs) with poly (3,4-ethylenedioxythiophene):poly (styrene sulfonate) (PEDOT:PSS), forming a choline chloride─acrylic acid─PEDOT:PSS (CAP) conductor with conducting interpenetrating nanogel networks. The CAP conductor is stretchable and self-healable due to ionic hydrogen bonding between the CA DESs and desulfurized PEDOT moieties. After treatment with sulfuric acid, structural rearrangement boosted the electrical conductivity of CAP by more than 100 times, achieving fast signal responses at high stretch─release rates and long-term anti-fatigue. Desulfurized CAP can realize a multifunctional smart wearable sensor.

Original language	English
Article number	110299
Journal	Composites Part B: Engineering
Volume	247
DOIs	https://doi.org/10.1016/j.compositesb.2022.110299
Publication status	Published - 2022 Dec

Bibliographical note

Publisher Copyright:
© 2022

Keywords

Damage tolerance
Electrical and mechanical properties
Nano-structures
Smart materials
Stretchable conductor

ASJC Scopus subject areas

Ceramics and Composites
Mechanics of Materials
Mechanical Engineering
Industrial and Manufacturing Engineering

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10.1016/j.compositesb.2022.110299

Cite this

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title = "Highly sensitive and long-term stretchable eutectic nanogel conductor with conducting interpenetrating nanogel networks for monitoring human motions",

abstract = "As a stretchable e-skin for sensing repetitive and stressful body movements, we photo-polymerized choline chloride─acrylic acid (CA) deep eutectic solvents (DESs) with poly (3,4-ethylenedioxythiophene):poly (styrene sulfonate) (PEDOT:PSS), forming a choline chloride─acrylic acid─PEDOT:PSS (CAP) conductor with conducting interpenetrating nanogel networks. The CAP conductor is stretchable and self-healable due to ionic hydrogen bonding between the CA DESs and desulfurized PEDOT moieties. After treatment with sulfuric acid, structural rearrangement boosted the electrical conductivity of CAP by more than 100 times, achieving fast signal responses at high stretch─release rates and long-term anti-fatigue. Desulfurized CAP can realize a multifunctional smart wearable sensor.",

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AU - Lim, Jun Ho

AU - Kim, Min Jeong

AU - Yoon, Ho Gyu

AU - Kim, Sang Woo

PY - 2022/12

Y1 - 2022/12

N2 - As a stretchable e-skin for sensing repetitive and stressful body movements, we photo-polymerized choline chloride─acrylic acid (CA) deep eutectic solvents (DESs) with poly (3,4-ethylenedioxythiophene):poly (styrene sulfonate) (PEDOT:PSS), forming a choline chloride─acrylic acid─PEDOT:PSS (CAP) conductor with conducting interpenetrating nanogel networks. The CAP conductor is stretchable and self-healable due to ionic hydrogen bonding between the CA DESs and desulfurized PEDOT moieties. After treatment with sulfuric acid, structural rearrangement boosted the electrical conductivity of CAP by more than 100 times, achieving fast signal responses at high stretch─release rates and long-term anti-fatigue. Desulfurized CAP can realize a multifunctional smart wearable sensor.

AB - As a stretchable e-skin for sensing repetitive and stressful body movements, we photo-polymerized choline chloride─acrylic acid (CA) deep eutectic solvents (DESs) with poly (3,4-ethylenedioxythiophene):poly (styrene sulfonate) (PEDOT:PSS), forming a choline chloride─acrylic acid─PEDOT:PSS (CAP) conductor with conducting interpenetrating nanogel networks. The CAP conductor is stretchable and self-healable due to ionic hydrogen bonding between the CA DESs and desulfurized PEDOT moieties. After treatment with sulfuric acid, structural rearrangement boosted the electrical conductivity of CAP by more than 100 times, achieving fast signal responses at high stretch─release rates and long-term anti-fatigue. Desulfurized CAP can realize a multifunctional smart wearable sensor.

KW - Damage tolerance

KW - Electrical and mechanical properties

KW - Nano-structures

KW - Smart materials

KW - Stretchable conductor

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ER -

Highly sensitive and long-term stretchable eutectic nanogel conductor with conducting interpenetrating nanogel networks for monitoring human motions

Abstract

Bibliographical note

Keywords

ASJC Scopus subject areas

Access to Document

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