Mercerization to enhance flexibility and electromechanical stability of reduced graphene oxide cotton yarns

Yong Ju Yun, Hyun Joo Lee, Tae Hyeong Son, Hyeontae Son, Yongseok Jun

Research output: Contribution to journalArticlepeer-review

15 Citations (Scopus)


Graphene-based textiles combining reduced graphene oxide (RGO) nanosheets and cotton textiles such as cotton yarns (CYs) and cotton fabrics show promise as multifunctional electronic textiles (e-textiles) that can be fabricated at reasonable cost by a simple solution process. However, realizing e-textiles with high flexibility and excellent mechanical stability is still challenging. Here, we report a facile strategy for the fabrication of highly flexible and electromechanically stable graphene yarns composed of RGO nanosheets and CYs. More specifically, the fully conformal wrapping of RGO sheets onto the surface of CYs is achieved by combination of conventional mercerization and simple dipping. We optimized the surface chemistry, morphology, and elasticity of the CYs as substrates by conventional mercerization. Using the obtained mercerized CYs, which had a more hydrated surface, round shape, smooth morphology, and good elasticity, we successfully fabricated high-quality graphene yarns. We evaluated the electrical and electromechanical behavior of the RGO-coated mercerized cotton yarns for e-textile and wearable applications. They exhibited a good electrical conductivity of ∼1.0 S/cm, which is approximately 1,000 times that of RGO-coated CYs without mercerization, and exceptional flexibility and electromechanical stability under 50,000 bending cycles with a maximum bending radius of 0.5 mm. We successfully demonstrated the potential application of our novel graphene yarns as wearable electronics with a fire/flame sensor. We believe that our process offers an easy approach to improve the flexibility and electromechanical reliability of two-dimensional nanomaterial-based cotton textiles such as fiber, yarn, and fabric than those that might be expected in advanced e-textiles and wearable devices.

Original languageEnglish
Article number107845
JournalComposites Science and Technology
Publication statusPublished - 2019 Nov 10

Bibliographical note

Funding Information:
Funding: This research was supported by the Basic Science Research Program through the National Research Foundation of Korea funded by the Ministry of Education ( 2018R1D1A1B07045581 ) and by the Ministry of Trade, Industry and Energy and the Korea Institute for Advancement of Technology through the International Cooperative R&D program (No. P006900001 ). This research was also supported by the KU Research Professor Program of Konkuk University.

Publisher Copyright:
© 2019 Elsevier Ltd


  • Coating
  • Durability
  • Electrical properties
  • Fibres
  • Flexible composites

ASJC Scopus subject areas

  • Ceramics and Composites
  • General Engineering


Dive into the research topics of 'Mercerization to enhance flexibility and electromechanical stability of reduced graphene oxide cotton yarns'. Together they form a unique fingerprint.

Cite this