The emerging covalent organic frameworks (COFs) for solar-driven fuels production

  • Changlei Xia
  • , Kent O. Kirlikovali
  • , Thi Hong Chuong Nguyen
  • , Xuan Cuong Nguyen
  • , Quoc Ba Tran
  • , Minh Khoa Duong
  • , Minh Tuan Nguyen Dinh
  • , Dang Le Tri Nguyen
  • , Pardeep Singh
  • , Pankaj Raizada
  • , Van Huy Nguyen
  • , Soo Young Kim
  • , Laxman Singh
  • , Chinh Chien Nguyen*
  • , Mohammadreza Shokouhimehr
  • , Quyet Van Le
  • *Corresponding author for this work

Research output: Contribution to journalReview articlepeer-review

Abstract

Photocatalysis-driven fuel production has garnered increasing attention as it can potentially address current energy- and environmental-related issues of the 21st century. However, the current performance of materials used for this application is still limited due to poor light absorption, fast photogenerated electron-hole recombination, and inappropriate active sites. Covalent organic frameworks (COFs), which offer an excellent platform to construct unique photocatalytic systems, have emerged as potential materials for the production of solar fuels. In this review, we investigate the development of COFs for three primary solar-driven fuel production strategies: (i) hydrogen (H2) production, (ii) carbon dioxide (CO2) reduction, and (iii) dinitrogen (N2) fixation. This review provides a roadmap to design excellent COF-based photocatalysts and highlights current limitations in the field of photocatalysis.

Original languageEnglish
Article number214117
JournalCoordination Chemistry Reviews
Volume446
DOIs
Publication statusPublished - 2021 Nov 1

Bibliographical note

Publisher Copyright:
© 2021 Elsevier B.V.

Keywords

  • Covalent organic frameworks
  • Fuel production
  • Photocatalysis

ASJC Scopus subject areas

  • Physical and Theoretical Chemistry
  • Inorganic Chemistry
  • Materials Chemistry

Fingerprint

Dive into the research topics of 'The emerging covalent organic frameworks (COFs) for solar-driven fuels production'. Together they form a unique fingerprint.

Cite this