Wide-Bandgap Metal Halide Perovskites for Tandem Solar Cells

Jinhui Tong, Qi Jiang, Fei Zhang, Seok Beom Kang, Dong Hoe Kim, Kai Zhu

Research output: Contribution to journalReview articlepeer-review

121 Citations (Scopus)

Abstract

Metal halide perovskite solar cells (PSCs) have become the most promising new-generation solar cell technology. To date, perovskites also represent the only polycrystalline thin-film absorber technology that has enabled >20% efficiency for wide-bandgap solar cells, making wide-bandgap PSCs uniquely positioned to enable high-efficiency and low-cost tandem solar cell technologies by coupling wide-bandgap perovskites with low-bandgap absorbers. In this Focus Review, we highlight recent research progress on developing wide-bandgap PSCs, including the key mechanisms associated with efficiency loss and instability as well as strategies for overcoming these challenges. We also discuss recent accomplishments and research trends on using wide-bandgap PSCs in perovskite-based tandem configurations, including perovskite/perovskite, perovskite/Si, perovskite/CIGS, and other emerging tandem technologies.

Original languageEnglish
Pages (from-to)232-248
Number of pages17
JournalACS Energy Letters
Volume6
Issue number1
DOIs
Publication statusPublished - 2021 Jan 8
Externally publishedYes

Bibliographical note

Funding Information:
The work at the National Renewable Energy Laboratory was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with Alliance for Sustainable Energy, Limited Liability Company (LLC), the Manager and Operator of the National Renewable Energy Laboratory. We acknowledge the support from the Derisking Halide Perovskite Solar Cells program of the National Center for Photovoltaics, funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Solar Energy Technologies Office. The views expressed in the article do not necessarily represent the views of the DOE or the U.S. Government. D.H.K and S.B.K. acknowledge the support by Korea Electric Power Corportaion (Grant Number: 20200528) and the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology (2019M3D1A2104109).

Publisher Copyright:
© 2021 American Chemical Society. All rights reserved.

ASJC Scopus subject areas

  • Chemistry (miscellaneous)
  • Renewable Energy, Sustainability and the Environment
  • Fuel Technology
  • Energy Engineering and Power Technology
  • Materials Chemistry

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